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Melting Of Al By Ultrafast Laser Pulses: Dynamics At The Melting Threshold

Melting Of Al By Ultrafast Laser Pulses: Dynamics At The Melting Threshold
Yudi Rosandi, Herbert M. Urbassek
Universitas Padjadjaran, Applied Physics A March 2013, Volume 110, Issue 3, pp 649–654, Publisher Name Springer-Verlag, Print ISSN 0947-8396, Online ISSN 1432-0630, https://doi.org/10.1007/s00339-012-7145-6
Bahasa Inggris
Universitas Padjadjaran, Applied Physics A March 2013, Volume 110, Issue 3, pp 649–654, Publisher Name Springer-Verlag, Print ISSN 0947-8396, Online ISSN 1432-0630, https://doi.org/10.1007/s00339-012-7145-6

Using molecular-dynamics simulation, we investigate the melting of a thin Al slab by ultrafast laser irradiation. We employ a laser energy, which is just around the melting threshold. While the equilibrium electron–phonon coupling is well understood, we investigate the in?uence of the early (i.e., prior to electron thermalization) electronlattice energy transfer. To this end, as a model study, we vary the fraction of the laser energy, which is directly given to lattice atoms vs. that given to the electronic system. We ?nd that the melting process depends sensitively on the early electron-lattice heating rate. The pressure build-up within the still solid parts of the slab is identified as the main agent which delays the melting transition. The changes in the simulated structure factor data suggest that X-ray measurements of thin ?lms performed just around the melting transition—even if performed long after electron thermalization—may provide information on the early electron-lattice energy coupling process.

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